Sensitivity of Atmospheric Carbon Dioxide to Dust Iron Solubility During the Last Glacial-Interglacial Cycle

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dc.catalogadorgjm
dc.contributor.authorOpazo Cuevas, Natalia Estefanía
dc.contributor.authorCosentino, Nicolás J.
dc.contributor.authorRidgwell, Andy
dc.contributor.authorLambert, Fabrice
dc.date.accessioned2025-03-12T19:22:36Z
dc.date.available2025-03-12T19:22:36Z
dc.date.issued2025
dc.description.abstractIron (Fe) input into remote oceans strongly influences the effectiveness of the biological pump and atmospheric carbon dioxide (CO2atm). Several pathways contribute to the delivery of Fe to the ocean surface, with mineral dust aerosols being fundamental beyond continental margins. The greatest variability in dust emissions occurs at glacial-interglacial timescales. While the absolute amount of dust is important, another key variable is the amount of soluble Fe within dust particles. However, the effect of this variable on past ocean biogeochemistry is not well documented by observations. Using the cGENIE Earth system model, we conducted sensitivity simulations of the role of dust-borne soluble Fe ocean inputs on the pre-industrial and Last Glacial Maximum (LGM) global CO2atm concentration. We found that the progressive enhancement of dust-borne Fe deposition and solubility in glacial oceans led to enhanced biological productivity. This shift in nutrient dynamics contributed to a 28% increase in global particulate organic carbon export. The resulting nonlinear reduction in LGM CO2atm (compared to the Holocene) increases up to a saturation value of ~30 ppmv, approximately one-third of the documented 80-100 ppmv change in CO2atm between glacial and interglacial periods during the late Quaternary. The region between 35ºS and the transition between the Subantarctic and Polar Fronts is particularly critical for regulating CO2atm. These results provide new insights into the role of Fe solubility in oceanic carbon fixation, emphasizing the need for a more complete understanding of dust particle mineralogy and its interactions with atmospheric and ocean chemistry in past and future climates.
dc.format.extent33 páginas
dc.fuente.origenORCID
dc.identifier.doi10.22541/essoar.173939611.14892129/v1
dc.identifier.urihttps://doi.org/10.22541/essoar.173939611.14892129/v1
dc.identifier.urihttps://repositorio.uc.cl/handle/11534/102542
dc.information.autorucInstituto de Geografía; Opazo Cuevas, Natalia Estefanía; S/I; 1031873
dc.information.autorucInstituto de Geografía; Lambert, Fabrice; 0000-0002-2192-024X; 250043
dc.language.isoen
dc.nota.accesocontenido parcial
dc.revistaESS Open Archive
dc.rightsacceso restringido
dc.subjectOceanography
dc.subjectBiogeochemistry
dc.subjectCarbon cycle
dc.subjectDust
dc.subjectEarth system model
dc.subjectPaleoceanography
dc.subject.ddc550
dc.subject.deweyCiencias de la tierraes_ES
dc.subject.ods06 Clean water and sanitation
dc.subject.ods13 Climate action
dc.subject.ods14 Life below water
dc.subject.odspa06 Agua limpia y saneamiento
dc.subject.odspa13 Acción por el clima
dc.subject.odspa14 Vida submarina
dc.titleSensitivity of Atmospheric Carbon Dioxide to Dust Iron Solubility During the Last Glacial-Interglacial Cycle
dc.typepreprint
sipa.codpersvinculados1031873
sipa.codpersvinculados250043
sipa.trazabilidadORCID;2025-03-03
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