Recent Advances of Fe-N-C pyrolyzed catalysts for the oxygen reduction reaction

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dc.contributor.authorMuñoz Becerra, Karina
dc.contributor.authorVenegas Toledo, Ricardo Alberto
dc.contributor.authorDuque, Luis
dc.contributor.authorZagal, José Heráclito
dc.contributor.authorRecio Cortés, Francisco Javier
dc.date.accessioned2021-12-02T12:58:27Z
dc.date.available2021-12-02T12:58:27Z
dc.date.issued2020
dc.description.abstractThis review summarizes recent advances in the development of pyrolyzed M–N–C catalysts for the oxygen reduction reaction, focusing on activity, stability, and the reactivity descriptors proposed for the rational design of pyrolyzed M–N–C catalysts. We discuss the last advances in achieving high catalytic activity and stability and the new insights into the characterization of FeN4 active sites by Mössbauer spectroscopy in combination with Density Functional Theory (DFT) calculations of the Fe–N–C catalysts. In addition, we present the different reactivity descriptors proposed in the literature for the rational design of Fe–N–C pyrolyzed materials: (i) structural descriptors determined by X-Ray Photoelectron Spectroscopy (XPS) and Mössbauer spectroscopy and (ii) the redox potential of the active center MNx.
dc.fuente.origenORCID
dc.identifier.doi10.1016/j.coelec.2020.08.006
dc.identifier.eissn2451-9103
dc.identifier.urihttps://doi.org/10.1016/j.coelec.2020.08.006
dc.identifier.urihttps://www.doi.org/10.1016/j.coelec.2020.08.006
dc.identifier.urihttps://repositorio.uc.cl/handle/11534/62997
dc.information.autorucEscuela de química ; Muñoz Becerra, Karina Massiel ; 0000-0001-9882-6342 ; 1033001
dc.information.autorucEscuela de química ; Venegas Toledo, Ricardo Alberto ; 0000-0001-7440-484X ; 1033002
dc.information.autorucEscuela de química ; Recio Cortés, Francisco Javier ; 0000-0002-5181-3197 ; 250556
dc.language.isoen
dc.nota.accesoContenido completo
dc.pagina.final161
dc.pagina.inicio154
dc.provenancengjara 2021-12-02 09:58:27
dc.relation.isformatofCurrent Opinion in Electrochemistry, vol. 23 (oct. 2020), pp. 154-161.
dc.revistaCurrent Opinion in Electrochemistry
dc.rightsacceso abierto
dc.subjectPyrolyzed M-N-C catalysts
dc.subjectOxygen reduction reaction
dc.subjectReactivity descriptors
dc.subjectMössbauer spectroscopy
dc.subjectRedox potential
dc.subject.ddc510
dc.subject.deweyMatemática física y químicaes_ES
dc.subject.otherFísica y química
dc.titleRecent Advances of Fe-N-C pyrolyzed catalysts for the oxygen reduction reaction
dc.typeartículo de revisión
dc.volumenVol. 23
sipa.codpersvinculados1033001
sipa.codpersvinculados1033002
sipa.codpersvinculados250556
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